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Journal Articles

Study of quasielastic barrier distributions as a step towards the synthesis of superheavy elements with hot fusion reactions

Tanaka, Taiki*; Morita, Kosuke*; Morimoto, Koji*; Kaji, Daiya*; Haba, Hiromitsu*; Boll, R. A.*; Brewer, N. T.*; Van Cleve, S.*; Dean, D. J.*; Ishizawa, Satoshi*; et al.

Physical Review Letters, 124(5), p.052502_1 - 052502_6, 2020/02

 Times Cited Count:19 Percentile:81.08(Physics, Multidisciplinary)

Journal Articles

Estimation of porosity and void fraction profiles in a packed bed of spheres using X-ray radiography

Ito, Daisuke*; Ito, Kei*; Saito, Yasushi*; Aoyagi, Mitsuhiro; Matsuba, Kenichi; Kamiyama, Kenji

Nuclear Engineering and Design, 334, p.90 - 95, 2018/08

 Times Cited Count:9 Percentile:62.99(Nuclear Science & Technology)

Two-phase flow through porous media must be well understood to develop a severe accident analysis code not only for light water reactor but also sodium-cooled fast reactor. When a core disruptive accident occurs in sodium-cooled fast reactor, the fuel inside the core become melted and interacts with the coolant. As a result, gas-liquid two-phase flow will be formed in the debris bed, which may have porous nature depending on the cooling process. In such condition, the local porosity and its distribution are very important to characterize two-phase flow field in the porous media. In this study, X-ray radiography was applied to measure the local porosity in the packed bed of spheres. The radial profiles were estimated from the chordal profiles measured by the X-ray method and compared with the previous porosity model. In addition, the void fraction radial profiles were also obtained in air-water two-phase flow.

Journal Articles

Characteristics and formation process of fractures in crystalline rocks in northern Kyushu

Murakami, Hiroaki; Ashizawa, Masaomi*; Tanaka, Kazuhiro*

Oyo Chishitsu, 59(1), p.2 - 12, 2018/04

This study describes the features of fractures and their fillings along with the long-term behavior of their hydrogeological structures in an underground environment based on the results of a geological investigation conducted at an underground facility in northern Kyushu. Fractures were classified into five groups on the basis of fracture orientation: A, B, C, D, and low-angle groups. The genesis of all fractures is the cooling process of granodiorite pluton. Almost all of the water-conducting fractures are included in the B group. Because a number of fracture fillings in the B group are filled by prehnite and crushed fragments of epidote and quartz, the fractures in this group alternated sealing and re-opening. The fracture characteristics in the B group are follow as: accompanying many alteration halos, long trace length, and cutting off other fractures. These results indicate that fractures in the B group have possibly functioned as pathways for groundwater flow in the long term.

JAEA Reports

Waste acceptance criteria for waste packages destined for near surface disposal containing radioactive waste from research, industrial and medical facilities; Study on a method that fills voidage in waste package with sandy soil

Nakata, Hisakazu; Hayashi, Hirokazu; Amazawa, Hiroya; Sakai, Akihiro

JAEA-Technology 2017-031, 41 Pages, 2018/01

JAEA-Technology-2017-031.pdf:5.27MB

JAEA plans to install disposal facilities for radioactive waste arising from research institutes. It must meet the technical standards specified in the relevant rule. One technical standard is that the disposal facilities shall be performance so as not to be left with the voids after the backfilling with soil. Additionally, the rule also requires this radioactive waste be enclosed in a container in which no harmful voids remain. In order to contribute to the development of a method that adapts the disposal facilities to these technical standards, JAEA adopts a waste conditioning artifice that aims for reducing a quantity of voidage in each waste container by a vibration filling method using sandy soil, providing with average void ratios inside the disposal facilities being adequately controlled. In this reports, filling property tests are conducted in the light of filling sand characteristics, types of metal waste and vibration conditions.

Journal Articles

Production of $$^{88}$$Nb and $$^{170}$$Ta for chemical studies of element 105, Db, using the GARIS gas-jet system

Huang, M.*; Haba, Hiromitsu*; Murakami, Masashi*; Asai, Masato; Kaji, Daiya*; Kanaya, Jumpei*; Kasamatsu, Yoshitaka*; Kikunaga, Hidetoshi*; Kikutani, Yuki*; Komori, Yukiko*; et al.

Journal of Radioanalytical and Nuclear Chemistry, 304(2), p.845 - 849, 2015/05

 Times Cited Count:3 Percentile:25.85(Chemistry, Analytical)

A technique to utilize radioisotopes of Nb and Ta was developed for chemical studies of element 105, Db, by coupling a gas-jet transport system to the RIKEN gas-filled recoil ion separator (GARIS). The short-lived $$^{88}$$Nb and $$^{170}$$Ta were produced with nuclear reactions using a $$^{19}$$F beam whose energy was the same as that to produce $$^{262}$$Db. Then, they were separated with GARIS and extracted to a chemistry laboratory with the gas-jet transport system. By changing only magnetic field of GARIS and inserting an energy degrader and a shutter for recoil ions, we could deliver the $$^{88}$$Nb and $$^{170}$$Ta to a chemistry device for $$^{262}$$Db without changing other experimental conditions.

Journal Articles

Magnetic and orbital fluctuations in filled skutterudites

Hotta, Takashi

Physica B; Condensed Matter, 378-380, p.51 - 53, 2006/05

 Times Cited Count:4 Percentile:22.76(Physics, Condensed Matter)

In order to clarify what types of spin and orbital fluctuations dominate over low-temperature electronic properties of Pr-based filled skutterudites, we evaluate multipole susceptibility based on a multiorbital Anderson model constructed from a $$j$$-$$j$$ coupling scheme. It is found that magnetic and quadrupole fluctuations are dominant at low temperatures. When we further include the effect of rattling as dynamical Jahn-Teller phonons, there remain quadrupole and octupole fluctuations, which may induce exotic superconducting pairing.

Journal Articles

Quasi-Kondo phenomenon due to the dynamical Jahn-teller effect

Hotta, Takashi

Physical Review Letters, 96(19), p.197201_1 - 197201_4, 2006/05

 Times Cited Count:40 Percentile:81.37(Physics, Multidisciplinary)

A mechanism of non-magnetic Kondo effect is proposed on the basis of a multiorbital Anderson model coupled with dynamical Jahn-Teller (JT) phonons. An electron system coupled dynamically with JT phonons has a vibronic ground state with double degeneracy due to clockwise and anti-clockwise rotational modes with entropy of $$log 2$$. When a temperature is lower than a characteristic energy to turn the rotational direction, the rotational degree of freedom is eventually suppressed and the corresponding entropy $$log 2$$ is released, leading to quasi-Kondo behavior. We discuss possible relevance of this quasi-Kondo phenomenon to electronic properties of filled skutterudites.

Journal Articles

Multipole fluctuations in filled skutterudites

Hotta, Takashi

Journal of the Physical Society of Japan, 74(9), p.2425 - 2429, 2005/09

 Times Cited Count:26 Percentile:73.62(Physics, Multidisciplinary)

In order to clarify exotic multipole properties of filled skutterudites, we evaluate multipole susceptibility for $$n$$=1$$sim$$5, where $$n$$ is the local $$f$$-electron number, on the basis of a multiorbital Anderson model constructed using the $$j$$-$$j$$ coupling scheme. For $$n$$=1, magnetic fluctuations dominate over low-temperature electronic properties, while for $$n$$=2 and 4, electronic states are dominated by both magnetic and quadrupole fluctuations. For $$n$$=3 and 5, octupole fluctuations are found to be significant, depending on the crystalline electric field potential. We discuss possible relevance of the results to actual materials.

Journal Articles

Microscopic approach to magnetism and superconductivity of $$f$$-electron systems with filled skutterudite structure

Hotta, Takashi

Journal of the Physical Society of Japan, 74(4), p.1275 - 1288, 2005/04

 Times Cited Count:25 Percentile:72.91(Physics, Multidisciplinary)

In order to understand electronic properties of filled skutterudite materials, the Anderson model is analyzed by using the numerical renormalization group method to evaluate magnetic susceptibility and entropy of $$f$$ electron for each case of $$n$$=1$$sim$$13, where $$n$$ is the number of $$f$$ electrons per rare-earth ion. For the $$f^2$$-electron system corresponding to the Pr-based filled skutterudite, it is found that magnetic fluctuations significantly remain at low temperatures, even when the ground state is $$Gamma_1$$ singlet, if $$Gamma_4^{(2)}$$ triplet is the excited state with small excitation energy. By analyzing an orbital degenerate Hubbard model constructed based on the $$j$$-$$j$$ coupling scheme, we find that anisotropic Cooper-pair mediated by magnetic fluctuations appears in a limited region in which the singlet and triplet ground states are interchanged.

JAEA Reports

Examination on detaching method of an irradiated mock-up with Li$$_{2}$$TiO$$_{3}$$ pebble bed from the core of JMTR

Ikeshima, Yoshiaki; Ishida, Takuya*; Tsuchiya, Kunihiko; Tomita, Kenji; Ebisawa, Hiroyuki; Magome, Hirokatsu; Nakamichi, Masaru*; Kitajima, Toshio; Kawamura, Hiroshi

JAERI-Tech 2005-005, 37 Pages, 2005/02

JAERI-Tech-2005-005.pdf:7.59MB

no abstracts in English

Journal Articles

Magnetic fluctuations of filled skutterudites emerging in the transition region between singlet and triplet states

Hotta, Takashi

Physical Review Letters, 94(6), p.067003_1 - 067003_4, 2005/02

 Times Cited Count:15 Percentile:62.72(Physics, Multidisciplinary)

In order to clarify magnetic properties of filled skutterudites, we analyze the Anderson model including seven $$f$$ orbitals hybridized with an $$a_{rm u}$$ conduction band using a numerical technique. For $$n$$=2 corresponding to Pr-based filled skutterudites, where $$n$$ is the local $$f$$-electron number, even if the ground state is a singlet, there remain significant magnetic fluctuations from a triplet state with a small excitation energy. This result can be understood by the fact that $$f$$-electron states are clearly distinguished as itinerant and localized ones in the filled skutterudite structure. This picture also explains the complex results for $$f$$-electron magnetic susceptibility and entropy for $$n$$=1$$sim$$13.

Journal Articles

$$^{31}$$P-NMR study of the uranium-based filled skutterudite compound UFe$$_4$$P$$_{12}$$

Tokunaga, Yo; Matsuda, Tatsuma; Sakai, Hironori; Kato, Harukazu*; Kambe, Shinsaku; Walstedt, R. E.; Haga, Yoshinori; Onuki, Yoshichika; Yasuoka, Hiroshi

Physical Review B, 71(4), p.045124_1 - 045124_5, 2005/01

 Times Cited Count:10 Percentile:42.74(Materials Science, Multidisciplinary)

$$^{31}$$P NMR measurements have been performed on the uranium-based ferromagnetic insulator UFe$$_4$$P$$_{12}$$ with $$T_C= 3.15$$ K. The field-orientation dependence of the hyperfine interaction has been measured using a single crystal, and the results compared with a point-dipolar field calculation assuming local moments at the U sites. We have also measured the field and temperature dependence of the nuclear spin-lattice relaxation rate ($$1/T_1$$) in several fields between 1.0 and 5.5 T at temperatures between 1.4 and 300 K. The results are discussed on the basis of a localized picture for the uranium 5f electrons.

Journal Articles

Super heavy elements

Koura, Hiroyuki

Uchu, 21(10), p.4 - 9, 2005/01

no abstracts in English

Journal Articles

Design and technology development of solid breeder blanket cooled by supercritical water in Japan

Enoeda, Mikio; Kosaku, Yasuo; Hatano, Toshihisa; Kuroda, Toshimasa*; Miki, Nobuharu*; Homma, Takashi; Akiba, Masato; Konishi, Satoshi; Nakamura, Hirofumi; Kawamura, Yoshinori; et al.

Nuclear Fusion, 43(12), p.1837 - 1844, 2003/12

 Times Cited Count:101 Percentile:93.45(Physics, Fluids & Plasmas)

no abstracts in English

Journal Articles

Thermal conductivity of neutron irradiated Be$$_{12}$$Ti

Uchida, Munenori*; Ishitsuka, Etsuo; Kawamura, Hiroshi

Fusion Engineering and Design, 69(1-4), p.499 - 503, 2003/09

 Times Cited Count:26 Percentile:82.89(Nuclear Science & Technology)

no abstracts in English

Journal Articles

Evaluation of effective thermal diffusivity of Li$$_2$$TiO$$_3$$ pebble bed under neutron irradiation

Kawamura, Hiroshi; Kikukawa, Akihiro*; Tsuchiya, Kunihiko; Yamada, Hirokazu*; Nakamichi, Masaru; Ishitsuka, Etsuo; Enoeda, Mikio; Ito, Haruhiko

Fusion Engineering and Design, 69(1-4), p.263 - 267, 2003/09

 Times Cited Count:3 Percentile:25.79(Nuclear Science & Technology)

no abstracts in English

Journal Articles

Effective thermal conductivity of a Li$$_{2}$$TiO$$_{3}$$ pebble bed for a demo blanket

Hatano, Toshihisa; Enoeda, Mikio; Suzuki, Satoshi; Kosaku, Yasuo; Akiba, Masato

Fusion Science and Technology, 44(1), p.94 - 98, 2003/07

 Times Cited Count:24 Percentile:81.86(Nuclear Science & Technology)

no abstracts in English

Journal Articles

Resonant X-ray scattering study on the filled skutterudite PrFe$$_4$$P$$_{12}$$

Ishii, Kenji; Inami, Toshiya; Murakami, Yoichi; Hao, L.*; Iwasa, Kazuaki*; Kogi, Masafumi*; Aoki, Yuji*; Sugawara, Hitoshi*; Sato, Hideyuki*; Imada, Shin*; et al.

Physica B; Condensed Matter, 329-333(1-4), p.467 - 468, 2003/05

 Times Cited Count:6 Percentile:35.62(Physics, Condensed Matter)

Resonant x-ray scattering study was carried out to investigate an anomalous ordered state ($$T_A$$ = 6.5 K) in the filled skutterudite PrFe$$_4$$P$$_{12}$$. At the Pr-$$L_{III}$$ absorption edge, we observed resonant features in $$h+k+l$$ = odd reflections, which are forbidden in the $$bcc$$ structure above $$T_A$$. Because these reflections contain the difference of anomalous scattering factor between two Pr atoms in the $$bcc$$ unit cell, and the ordered state is attributed to the ordering of two different electronic states of Pr.

Journal Articles

Development of a micro gas chromatograph for the analysis of hydrogen isotope gas mixtures in the fusion fuel cycle

Kawamura, Yoshinori; Konishi, Satoshi; Nishi, Masataka

Fusion Engineering and Design, 58-59, p.389 - 394, 2001/11

 Times Cited Count:26 Percentile:85.07(Nuclear Science & Technology)

no abstracts in English

Journal Articles

${it In-situ}$ tritium recovery experiments of blanket in-pile mockup with Li$$_{2}$$TiO$$_{3}$$ pebble bed in Japan

Tsuchiya, Kunihiko; Nakamichi, Masaru; Nagao, Yoshiharu; Enoeda, Mikio; Osaki, Toshio*; Tanaka, Satoru*; Kawamura, Hiroshi

Journal of Nuclear Science and Technology, 38(11), p.996 - 1003, 2001/11

 Times Cited Count:23 Percentile:82.42(Nuclear Science & Technology)

no abstracts in English

83 (Records 1-20 displayed on this page)